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Journal Articles

ALTEMIS: Using integrated hydrology and reactive transport modeling to support resilience at the Savannah River Site

Xu, Z.*; Litzinger, A.*; Sakuma, Kazuyuki; Arora, B.*; Hazenberg, P.*; Wang, L.*; Gonzalez Raymat, H.*; Fabricatore, E.*; Wainwright, Haruko*; Eddy-Dilek, C.*

Proceedings of Waste Management Symposia 2024 (WM2024) (Internet), 14 Pages, 2024/03

Journal Articles

Effectiveness of fused LASSO for prediction of distribution of radioactive materials in reactor buildings

Yamada, Susumu; Yoshida, Toru*; Hasegawa, Yukihiro*; Machida, Masahiko

Proceedings of Waste Management Symposia 2024 (WM2024) (Internet), 15 Pages, 2024/03

In order to safely carry out the decommission of reactor buildings, it is extremely important to identify the radiation source distribution. It has been reported that when the structural model of the building is constructed by uniform cells, the source distribution can be estimated from the measured air dose rates by minimizing an evaluation function using the Least Absolute Shrinkage and Selection Operator (LASSO). Moreover, if cells are non-uniform, we can estimate the distribution using the fused LASSO which minimizes the evaluation function that takes account of the connectivity between the adjacent cells. However, when a group of some cells is considered disconnected from the surrounding ones due to the precision of the measured structural data, the concentration of the group can be singularly high. Therefore, in order to avoid the problem, we propose a new evaluation function that can prevent the singularity. We estimated the distribution for the test model using the proposed evaluation function and confirmed the validity of the function. Moreover, we succeeded in estimating the source distribution in the pool canal circulation system room in JMTR in the Japan Atomic Energy Agency by the fused LASSO for the new function more accurately than previous analysis.

Journal Articles

Sorption behavior of niobium onto clay minerals in the presence of Ca

Ohira, Saki; Iida, Yoshihisa

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 10 Pages, 2023/02

The sorption distribution coefficient (${it K}$d) of niobium-94 (Nb-94) on minerals is one of the important parameters in safety assessment of radioactive waste disposal. In a previous study, the ${it K}$d values of Nb under alkali condition in the presence of Ca, were two orders of magnitude higher than those in the presence of Na. In this study, Nb sorption experiments were performed to reexamine the effect of Ca on Nb sorption on clay minerals, and blank tests were performed to check for precipitation formation. The results showed that the Nb sorption onto montmorillonite and illite, did not depend on the Ca concentration, and ${it K}$d values obtained in the presence of Ca were the same as those in the absence of Ca. A sorption model assuming sorption by complexation on the mineral surface was developed and then calculated using the geochemical calculation code. The model with the surface species X_ONb(OH)$$_{4}$$ and X_ONb(OH)$$_{5}$$$$^{-}$$ represented trends in the data obtained.

Journal Articles

Laboratory experiment on runoff of particles deposited on land surface by rainfall at accidents in the decommissioning stage

Shimada, Taro; Namekawa, Masakazu*; Miwa, Kazuji; Takeda, Seiji

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 8 Pages, 2023/02

It is supposed that radioactive dust deposited at the land surface will be moved downstream and concentrated at the depression by overland flow at heavy rain after the accidental release of radioactive dusts accumulated at the filters in the decommissioning stage of nuclear facilities. The authors are developing a calculation code to evaluate distribution changes of radioactivity on the surface and public dose considering the conditions such as rainfall, topography and types of cover surface. It is necessary to construct methods for setting parameter values used for the calculations based on the actual situation. Therefore, the parameter values were obtained by the experiments where Fe$$_3$$O$$_4$$ powder spread on the cover surface such as smooth and aged-asphalt, concrete and bare soil, was eroded by overland flow and raindrops and they were collected at the lower end of the slope at a minute interval. The collected weights of overland flow and Fe$$_3$$O$$_4$$ powder were measured. Based on the Manning's roughness coefficient for smooth asphalt already known as a fixed value, the erosion velocity coefficient was evaluated. Then Manning's roughness coefficients for other cover surfaces were obtained using the erosion velocity coefficient. Manning's roughness coefficients were slightly smaller than the range of literature values. In addition, elevations for the cover surface were measured by 3D scanner as point cloud data, and the surface roughness were evaluated. The values of surface roughness and Manning's roughness coefficients had a correlation. It indicated a possibility to utilize the surface roughness to set the Manning's roughness coefficient for the evaluation of radioactivity distribution change by heavy rainfall.

Journal Articles

LASSO reconstruction scheme to predict radioactive source distributions inside reactor building rooms; Theory & demonstration

Shi, W.*; Machida, Masahiko; Yamada, Susumu; Yoshida, Toru*; Hasegawa, Yukihiro*; Okamoto, Koji*

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 8 Pages, 2023/02

Journal Articles

LASSO reconstruction scheme to predict radioactive source distributions inside reactor building rooms; Practical applications

Machida, Masahiko; Shi, W.*; Yamada, Susumu; Miyamura, Hiroko; Yoshida, Toru*; Hasegawa, Yukihiro*; Okamoto, Koji; Aoki, Yuto; Ito, Rintaro; Yamaguchi, Takashi; et al.

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 11 Pages, 2023/02

Journal Articles

A Project focusing on the contamination mechanism of concrete after the accident at Fukushima Daiichi Nuclear Power Plant

Yamada, Kazuo*; Maruyama, Ippei*; Haga, Kazuko*; Igarashi, Go*; Aihara, Haruka; Tomita, Sayuri*; Kiran, R.*; Osawa, Norihisa*; Shibata, Atsuhiro; Shibuya, Kazutoshi*; et al.

Proceedings of International Waste Management Symposia 2021 (WM2021) (CD-ROM), 10 Pages, 2021/03

Journal Articles

New project on the analysis of contamination mechanisms of concrete at the Fukushima Daiichi Nuclear Power Station

Yamada, Kazuo*; Maruyama, Ippei*; Koma, Yoshikazu; Haga, Kazuko*; Igarashi, Go*; Shibuya, Kazutoshi*; Aihara, Haruka

Proceedings of International Waste Management Symposia 2019 (WM2019) (CD-ROM), 6 Pages, 2019/03

Journal Articles

Dose estimation in recycling of decontamination soil due to Fukushima NPS accident as coastal levees

Takai, Shizuka; Sawaguchi, Takuma; Takeda, Seiji

Proceedings of International Waste Management Symposia 2018 (WM2018) (Internet), 14 Pages, 2018/03

After the Fukushima Nuclear Power Station accident, large quantities of radiocesium-contaminated soil generated from decontamination activities have been stored in the Fukushima prefecture. To complete the final disposal of decontamination soil, the Ministry of the Environment of Japan presented policy to reduce the disposal volume by using low-level decontamination soil as recycled materials. The use will be limited to civil engineering structures in public projects, such as coastal levee and road embankment. However, there has been no example or safety assessment of recycling of decontamination soil. To contribute to guideline development for the recycling by the Ministry of the Environment, we conducted the safety assessment for recycling of decontamination soil as coastal levee. First, we evaluated additional doses to workers and the public in the case of construction and service of coastal levee. From the result, the radioactive cesium concentration level of recycled materials was derived to be 6,800 Bq/kg. For general designs of coastal levee in Japan, additional doses to the public in the case of service were below 0.01 mSv/y with derived radioactivity level. Finally, we confirmed additional doses in the case of disaster to be below 1 mSv/y.

Journal Articles

A Multiscale Bayesian data integration approach for mapping air dose rates around the Fukushima Daiichi Nuclear Power Plant

Wainwright, Haruko*; Seki, Akiyuki; Chen, J.*; Saito, Kimiaki

Proceedings of International Waste Management Symposia 2017 (WM2017) (Internet), 8 Pages, 2017/03

We integrate various types of datasets, such as ground-based walk and car surveys, and airborne surveys, all of which have different scales, resolutions, spatial coverage, and accuracy. This method is based on geostatistics to represent spatial heterogeneous structures, and also on Bayesian hierarchical models to integrate multiscale, multitype datasets in a consistent manner. The Bayesian method allows us to quantify the uncertainty in the estimates, and to provide the confidence intervals that are critical for robust decision-making. We showed the demonstration of Bayesian data integration approach for the Fukushima evacuation zones with high air dose rates.

Journal Articles

Computational and experimental examination of simulated core damage and relocation dynamics of a BWR fuel assembly

Hanus, G.*; Sato, Ikken; Iwama, Tatsuya*

Proceedings of International Waste Management Symposia 2016 (WM2016) (Internet), 12 Pages, 2016/03

JAEA plans a large-scale test to evaluate damage and relocation behavior of BWR core materials consisting of fuel rods, channel boxes, control blade and lower support structures. Its purpose is to contribute to understanding of core material relocation behavior in the event of severe accidents with the BWR design conditions for which existing experimental database is quite limited. Prior to large-scale testing, JAEA desires preliminary investigations to examine melting test pieces. The purpose of such tests is to verify the materials and test piece will be heated by plasma to the target temperature (ca.2900K) and to collect data about the material relocation behavior. Results from preliminary computational simulations are presented illustrating the effectiveness of a 150 kW non-transferred plasma jet. An experimental test program using the computational analyses as a basis and a plasma torch is described.

Journal Articles

Status and future plan of decommissioning of the Plutonium Fuel Fabrication Facility

Kuba, Meiji; Watahiki, Masatoshi; Hirano, Hiroshi; Ishikawa, Shinichiro; Sato, Hisato

Proceedings of International Waste Management Symposia 2014 (WM2014) (Internet), 12 Pages, 2014/05

Plutonium Fuel Fabrication Facility is now in a decommissioning phase. In the facility, stabilizing activities of nuclear material residuals remained and the gloveboxes dismantling activities have been carried out simultaneously. Glovebox dismantling activities are performed manually by a worker wearing air-feed suit with mechanical tools in a plastic enclosure which is constructed around the glove boxes for preventing spread of contamination. However, the mental load and physical load of the worker are intensively high. Therefore, worker's safely issue still exists and need to be resolved. Moreover, occupational time for the worker is restricted to only one hour per day, which in turn make shortening schedule and cost savings almost impossible. R&D of new dismantling methods including application of heavy equipment with anti-contamination measure to strengthen the work performance in the plastic enclosures has been started to reduce the above mentioned potential risks and costs.

Journal Articles

Release behavior of radioactive materials at a boiling accident of high active liquid waste in reprocessing plants

Uchiyama, Gunzo; Tashiro, Shinsuke; Amano, Yuki; Abe, Hitoshi; Yamane, Yuichi; Yoshida, Kazuo; Ishikawa, Jun

Proceedings of International Waste Management Symposia 2014 (WM2014) (Internet), 9 Pages, 2014/05

The experimental study for source term data of radioactive materials has been conducted at a boiling accident of high active liquid waste (HALW) in a reprocessing plant. In the small scale cold test using a non-radioactive simulated HALW, the release behavior of FP elements from the simulated HALW were investigated under various boiling accident conditions. In the engineering scale cold test, the release behavior of FP elements at boiling accident conditions was investigated mainly as a spatial function. In the small scale hot test using a radioactive simulated HALW, the release behavior of radioactive materials (FP, alpha nuclides) were obtained under typical boiling accident conditions. In the small scale hot test, the release fractions of Ru and non-volatile FPs obtained were almost the same as those of the small scale cold test.

Journal Articles

Adsorption of ruthenium, rhodium and palladium from simulated high-level liquid waste by highly functional xerogel

Onishi, Takashi; Koyama, Shinichi; Mimura, Hitoshi*

Proceedings of International Waste Management Symposia 2013 (WM2013) (CD-ROM), 7 Pages, 2013/02

As part of a development of nuclides separation process by using highly-functional xerogels, xerogels including insoluble ferrocyanide compounds were prepared for separation of Pt group metals. Adsorption and elution behaviors of Pt group metals were investigated in simulated high level radioactive liquid waste. Removal of sulfur from recovered palladium was also conducted by a thermal decomposition and digestion method.

Journal Articles

Study on evaluation of project management data for decommissioning of uranium refining and conversion plant

Usui, Hideo; Izumo, Sari; Shibahara, Yuji; Morimoto, Yasuyuki; Tokuyasu, Takashi; Takahashi, Nobuo; Tanaka, Yoshio; Sugitsue, Noritake; Tachibana, Mitsuo

Proceedings of International Waste Management Symposia 2012 (WM2012) (CD-ROM), 13 Pages, 2012/02

Dismantling of dry conversion facility in the uranium refining and conversion plant at Ningyo-toge began in 2008. During dismantling activities, project management data have been collected. Establishment of the calculation formula for dismantling of each kind of equipment makes it possible to evaluate manpower for dismantling the whole facility. However, it is not easy to prepare calculation formula for all kinds of equipment in the facility. Therefore, a simpler evaluation method was considered to calculate manpower based on facility characteristics. The results showed promise for evaluating dismantling manpower with respect to each chemical process. To create an effective dismantling plan, it is necessary to carefully consider use of a GH preliminarily. Thus, an evaluation method of project management data such as manpower and secondary waste generation was considered. The results showed promise for evaluating project management data of GH by using established calculation formula.

Journal Articles

Sensitivity analysis for scenarios relevant to evolution of overpack and buffer material

Takeda, Seiji; Watanabe, Masatoshi; Kimura, Hideo

Proceedings of International Waste Management Symposia 2011 (WM2011) (CD-ROM), 11 Pages, 2011/05

This study focuses on a deterioration of expected barrier functions relevant to evolution of overpack and sand-bentonite buffer material in engineered barrier system in the geological disposal of high-level radioactive waste. Release rates for important radionuclides, Cs-135 and Se-79, were estimated from Monte Carlo-based analysis for the early failure of overpack and the buffer alteration scenarios. One of the possible early failure scenarios is the change of glass dissolution rate, effective diffusion coefficients and distribution coefficients in the buffer material, which are affected by early high temperature in the engineered barrier. The analytical result indicates that this scenario has no detrimental effect on the maximum release rates of these radionuclides. Another scenario is the occurrence of the increase of Se solubility correlated with the enhanced redox potential due to the radiolysis after the early failure of overpack. This scenario allows a conspicuous increase in the maximum release rates of Se-79 from the buffer, which is over one order of magnitude higher than that in the normal scenario. In addition, with the comparison of the maximum release rates between the early failure scenario and the buffer alteration scenario, it is suggested that the effect of the deterioration of the expected barrier functions relevant to the buffer alteration on the release rates is more remarkable than the effect on early failure.

Journal Articles

Performance of steam reforming technology in a long term treatment of waste TBP/dodecane

Nakagawa, Akinori; Sone, Tomoyuki; Sasaki, Toshiki; Nakazawa, Osamu; Tashiro, Kiyoshi

Proceedings of International Waste Management Symposia 2011 (WM2011) (CD-ROM), 7 Pages, 2011/03

Journal Articles

Cement based encapsulation experiments for low-radioactive liquid waste at Tokai Reprocessing Plant

Sugaya, Atsushi; Tanaka, Kenji; Akutsu, Shigeru

Proceedings of International Waste Management Symposia 2011 (WM2011) (CD-ROM), 11 Pages, 2011/02

The main component of the liquid wastes is sodium nitrate. Nitrate ion decomposition technology is under development to conserve a circumference environment of a disposal site. To investigate the methods for decomposing nitrate ion, several small-scale trials were performed using reductants and a catalyst in sodium nitrate solutions. It will be reported that the cement based encapsulation trials to immobilize the sodium carbonate based liquid waste, which was performed under non-radioactive condition at both small and full scale to investigate the optimum cement formulation.

Journal Articles

Experiences of Remote Operated Dismantling of Glove-Box

Okada, Takashi; Asazuma, Shinichiro; Kashiro, Kashio; Matsumoto, Masaki

CD-ROM, WM-5214, p.8, 8 Pages, 2005/00

The dismantling activities, which consist of removal of the glove panel, dismantling of the interior equipment and dismantling of the GB body and made up about 45% of the dismantling of the GB in GBDF, could be performed by remote control.

Journal Articles

Application of modified truex flowsheet to minor actinide from high level liquid waste

Kawata, Tomio; ; Nomura, Kazunori; ;

WM Symposia, 0 Pages, 1993/00

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